Time-resolved
imaging of micrometer-scale phenomena in liquids
- Time-resolved
imaging of plasmonic nanoparticles in liquids (Sclieren
photography, shadowgraph & Mie scattering)
- Multi-phase
thermodynamics of heat conduction
- Spatially resolved visualization of ions in aqueous solutions
- Classical density functional theory of liquids
Research
Species with sizes less than the
diffraction limit cannot be visualized in liquids by direct
optical methods. We are developing new experimental methods for
determining positions and sizes of individual plasmonic
nanoparticles in the liquid phase by rapid laser heating. The heat
conduction within the multiphase system (particle-gas-liquid)
results in the production of gaseous bubbles around the particles,
which can be used to estimate their positions as well as their
sizes by thermodynamic modeling. Another application of the work
is to develop more accurate models for estimating heat delivery by
the particles, which is important for heat solar heat capture
applications and photothermal cancer treatment. Our current work
extends the previously developed techniques to visualize ionic
species in aqueous solutions together with the implementation of
classical density functional theory methods for describing the
dynamic response of the system.
Selected recent publications
Laser assisted detection of metal nanoparticles in liquid He-II,
V. Fernandez, A. Garcia, K. Vossoughian, E. Popov, S. Garrett, and
J. Eloranta. Journal of Physical Chemistry A 119, 10882
(2015).
Ejection of metal particles into superfluid 4He
by laser ablation, X. Buelna, A. Freund, D. Gonzalez, E.
Popov, and J. Eloranta. Journal of Physical Chemistry B 120,
11010 (2016).
Application of time-resolved shadowgraph imaging and computer
analysis to study micrometerscale response of superfluid helium,
S. Sajjadi, X. Buelna, and J. Eloranta. Review of Scientific
Instruments 89, 013102 (2018).
Time-resolved shadowgraph photography of laser-heated plasmonic
gold nanoparticles in water, D. Stavich, B. Nestoiter, D.
Gonzalez, A. Freund, X. Buelna, K. Wang, J. Teprovich, and J.
Eloranta. Journal of Physical Chemistry C 124, 14022 (2020).
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